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91.
92.
《Ceramics International》2020,46(17):26637-26645
Intense research work is underway for identifying materials with potential applications in energy storage and energy harvesting systems. The magnesium based scandium chalcogenides have recently emerged as potential candidates for Mg batteries owing to their high Mg ionic conductivity and low electron conduction. At the same time, their band gaps are capable of absorbing electromagnetic radiations in visible to UV range; making them suitable for solar cell applications. In order to analyze the application of MgSc2X4(X = S, Se) compounds in energy devices, in this work we employ density functional theory calculations using the full potential linear augmented plane-wave method for examining their optoelectronic and thermoelectric properties. For the structural properties, the generalized gradient approximation functional designed for solids (PBEsol-GGA) has been used, while modified Becke and Johnson (mBJ) potential functional is used for computing the optoelectronic and transport properties. Our calculated optical properties indicate that these materials can find applications in solar cells. Moreover, the electronic transport properties computed using Boltzmann transport equation suggest carrier concentrations in MgSc2S4 to MgSc2Se4 spinels can be tuned for making them suitable for metal ion batteries. 相似文献
93.
Akhilesh Raj Sarangapani Jagannathan Tansel Yucelen 《International Journal of Adaptive Control and Signal Processing》2020,34(3):330-353
Heterogeneous sensor networks (HSN) find a wide range of applications in the field of military and civilian environments, where sensor nodes are utilized to estimate the position of a target with both dynamics and control input being unknown for the purposes of tracking. In the HSN, nodes are considered active depending upon their ability to sense the target output while the others are taken passive. Accurate estimation requires local information exchange among the spatially located sensor nodes, so that the active nodes as well as the passive nodes converge simultaneously to the same value. The local information exchange among the nodes is dictated by a connected graph. By using the criterion of collective observability, a novel distributed adaptive estimation scheme is introduced via adaptive observer where the nodes are allowed to have different sensor modalities. Using the estimated information, a subset of active and passive nodes, referred to as mobile nodes, can track the moving target. By using a constant state feedback controller at each mobile node, the state and parameter estimation as well as the tracking errors are shown to be uniformly ultimately bounded. Simulation results verify theoretical claims. 相似文献
94.
The association between miRNA and disease has attracted more and more attention. Until now, existing methods
for identifying miRNA related disease mainly rely on top-ranked association model, which may not provide a full landscape
of association between miRNA and disease. Hence there is strong need of new computational method to identify the
associations from miRNA group view. In this paper, we proposed a framework, MDA-TOEPGA, to identify miRNAdisease association based on two-objective evolutionary programming genetic algorithm, which identifies latent miRNAdisease associations from the view of functional module. To understand the miRNA functional module in diseases, the
case study is presented. We have been compared MDA-TOEPGA with several state-of-the-art functional module
algorithm. Experimental results showed that our method cannot only outperform classical algorithms, such as K-means,
IK-means, MCODE, HC-PIN, and ClusterONE, but can also achieve an ideal overall performance in terms of a
composite score consisting of f1, Sensitivity, and Accuracy. Altogether, our study showed that MDA-TOEPGA is a
promising method to investigate miRNA-disease association from the landscapes of functional module. 相似文献
95.
《中国有色金属学会会刊》2022,32(5):1705-1717
In view of the unclear cause of perfluorocarbons (PFCs) emission in the anode effect stage of aluminum electrolysis, the microscopic formation mechanism of PFCs was studied by density functional theory calculation and X-ray photoelectron spectroscopy (XPS). It is found that the discharge of fluorine containing anions ([F]?) on carbon anode first causes the substitution of C—H by C—F and further results in the saturation of aromatic C—C bonds, leading to the appearance of —CF3 or —C2F5 group through six-carbon-ring opening. Elimination of —CF3 and —C2F5 with F atom could be a likely mechanism of CF4 and C2F6 formation. XPS results confirm that different types of —CFx group can be formed on anode surface during electrolysis, and the possibility that [F]? discharges continuously at the C edge and finally forms different C—F bonds in quantum mechanical calculation was verified. 相似文献
96.
《中国有色金属学会会刊》2022,32(12):4139-4155
Between the two major arsenic-containing salts in natural water, arsenite (As(III)) is far more harmful to human and the environment than arsenate (As(V)) due to its high toxicity and transportability. Therefore, preoxidation of As(III) to As(V) is considered to be an effective means to reduce the toxicity of arsenic and to promote the removal efficiency of arsenic. Due to their high catalytic activity and arsenic affinity, iron-based functional materials can quickly oxidize As(III) to As(V) in heterogeneous Fenton-like systems, and then remove As(V) from water through adsorption and surface coprecipitation. In this review, the effects of different iron-based functional materials such as zero-valent iron and iron (hydroxy) oxides on arsenic removal are compared, and the catalytic oxidation mechanism of As(III) in heterogeneous Fenton process is further clarified. Finally, the main challenges and opportunities faced by iron-based As(III) oxidation functional materials are prospected. 相似文献
97.
In this paper, a robust controller for a Six Degrees of Freedom (6 DOF) coaxial octorotor helicopter control is proposed in presence of actuator faults. Radial Base Function Neural Network (RBFNN), Fuzzy Logic Control approach (FLC) and Sliding Mode Control (SMC) technique are used to design a controller, named Fault Tolerant Control (FTC), for each subsystem of the octorotor helicopter. The proposed FTC scheme allows avoiding difficult modeling, attenuating the chattering effect of the SMC, reducing the rules number of the fuzzy controller, and guaranteeing the stability and the robustness of the system. The simulation results show that the proposed FTC can greatly alleviate the chattering effect, good tracking in presence of actuator faults. 相似文献
98.
M. Abbasnejad S.J. Azimi M.R. Mohammadizadeh 《International Journal of Hydrogen Energy》2018,43(3):1587-1595
Structural and electronic properties of complex hydride Mg(BH4)(NH2), applicable in hydrogen storage, were studied in framework of pseudopotential-density functional theory. This compound shows an indirect band gap of 4.95 eV which is categorized in insulator materials. The calculated total and partial density of states of this compound show that the hydrogen bonding in BH4 anion is mainly covalent and the hydrogen-hydrogen repulsion is more in anion BH4 than in anion NH2. The calculated bulk modulus from Birch-Murnaghan equation of state is in close agreement with that obtained from the elastic constants. The obtained bulk modulus (19.27 GPa) shows this compound is more ductile than binary and ternary hydrides and it does not have a brittle structure. Therefore, it is a good candidate for hydrogenation and dehydrogenation cycles. The stability of the structure in ambient pressure is also declared by calculating the elastic coefficients. However, the existence of elastic anisotropy in the compound demonstrates the less compressibility of it along the c axis than a and b axes. The small amount of Poisson ratio indicates that it is more stable against shear compared to common borohydrides. This point is important for hydride stability in hydrogenation and dehydrogenation cycles. 相似文献
99.
The long-established use of enzymes for food processing and product formulation has resulted in an increased enzyme market compounding to 7.0% annual growth rate. Advancements in molecular biology and recognition that enzymes with specific properties have application for industrial production of infant, baby and functional foods boosted research toward sourcing the genes of microorganisms for enzymes with distinctive properties. In this regard, functional metagenomics for extremozymes has gained attention on the premise that such enzymes can catalyze specific reactions. Hence, metagenomics that can isolate functional genes of unculturable extremophilic microorganisms has expanded attention as a promising tool. Developments in this field of research in relation to food sector are reviewed. 相似文献
100.
Theoretical investigation of anisotropic mechanical and thermal properties of ABO3 (A=Sr,Ba; B=Ti,Zr, Hf) perovskites 下载免费PDF全文
Yuchen Liu Bin Liu Huimin Xiang Yanchun Zhou Hongqiang Nian Hongfei Chen Guang Yang Yanfeng Gao 《Journal of the American Ceramic Society》2018,101(8):3527-3540
As promising TBC (thermal barrier coating) candidates, perovskite oxides own designable properties for their various options of cations and structural diversity, but limited comprehensions of structure‐property relationship delay their engineering applications. In this work, mechanical/thermal properties of ABO3 (A=Sr, Ba; B=Ti, Zr, Hf) perovskites and their anisotropic nature are predicted employing density functional theory. Their theoretical minimum thermal conductivities range from 1.09 to 1.74 W·m?1·K?1, being lower than Y2O3 partially stabilized ZrO2. Reduced thermal conductivities up to 16% along particular directions are reached after considering thermal conductivity anisotropy. All compounds own high hardness while SrZrO3, SrHfO3, and BaHfO3 possess well damage tolerance. We found that small electronegativity discrepancy leads to big anisotropy of chemical bond, Young's/shear moduli and thermal conductivities, together with good damage tolerance. These results suggest that the next generation TBCs with extra low thermal conductivity should be achieved through combining material design and orientation‐growth tailoring. 相似文献